Journal
CHEMICAL COMMUNICATIONS
Volume 52, Issue 62, Pages 9711-9714Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6cc04327e
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Funding
- National Natural Science Foundation of China [21476043, 21120102036, 21361130020]
- National Basic Research Program of China (973 program) [2014CB239402]
- Natural Science Foundation of Liaoning Province [2014020010]
- Swedish Energy Agency
- K & A Wallenberg Foundation
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Molecular ruthenium catalysts were found to selectively catalyze the oxidation of thioanisole to sulfoxide with a yield up to 100% in the presence of visible light and sacrificial reagents when they were anchored onto hematite powder. The composite photocatalysts also showed about 5 times higher efficiencies in benzyl alcohol oxidation than the system composed of dispersed molecular catalysts and hematite particles in aqueous solution. A photoelectrochemical cell based on a molecular catalyst modified hematite photoanode was further fabricated, which exhibited high activity towards the oxidation of organic substrates.
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