Journal
CHEMICAL COMMUNICATIONS
Volume 52, Issue 24, Pages 4485-4488Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6cc00930a
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Funding
- NSFC [21472167]
- Zhejiang Provincial NSFC [LR16B020001]
- Research Fund for the Doctoral Program of Higher Education of China [20120101120087]
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The first enantioselective total synthesis of (+)-alsmaphorazine E has been achieved through a traceless chirality transfer strategy, which also enabled structural reassignment of the natural product. Key features of this efficient approach entail a catalytic intramolecular oxidative cyclization, a diastereoselective oxidative cyclic aminal formation and a radical cyclization/transannular aza-Michael addition cascade.
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