Journal
CHEMICAL COMMUNICATIONS
Volume 52, Issue 77, Pages 11571-11574Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6cc06060a
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- Swedish Research Council VR
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In the context of green chemistry, the replacement of high molecular weight stoichiometric oxidants with O-2 is most desirable but difficult. Here, we report the asymmetric aerobic oxidative synthesis of dihydropyranones. The oxidation is aided by a system of electron transfer mediators and is selective toward the homoenolate. The dihydropyranones can be isolated in high to excellent yields, with high ee (up to 95%).
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