Journal
CHEMICAL COMMUNICATIONS
Volume 52, Issue 24, Pages 4462-4465Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cc10212j
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Funding
- NIGMS NIH HHS [R01 GM096000, R01 GM062248] Funding Source: Medline
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Solvent D2O and O-18 kinetic isotope effects on RNA 20-O-transphosphorylation catalyzed by Zn2+ demonstrate an altered transition state relative to specific base catalysis. A recent model from DFT calculations involving inner sphere coordination to the non-bridging and leaving group oxygens is consistent with the data.
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