Journal
CHEMICAL COMMUNICATIONS
Volume 52, Issue 85, Pages 12614-12617Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6cc06608a
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Funding
- National Natural Science Foundation of China [51402100, 21573066]
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Designing highly active, earth-abundant and stable bifunctional electrocatalysts for both the oxygen (OER) and hydrogen (HER) evolution reactions is very crucial to overall water splitting. Herein, we developed nanoparticle-stacked porous Co3FeNx (NSP-Co3FeNx) nanowires as bifunctional electrocatalysts, exhibiting excellent OER and HER activity with a low overpotential of 222 mV at 20 mA cm(-2) and 23 mV at 10 mA cm(-2), respectively, due to their unique structural advantages with grain boundaries, defects and dislocations. Moreover, the electrocatalysts as bifunctional electrodes show a high performance with 10 mA cm(-2) at a cell voltage of 1.539 V.
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