Journal
CHEMICAL COMMUNICATIONS
Volume 52, Issue 33, Pages 5753-5756Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6cc00766j
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Funding
- National Natural Science Foundation of China [21476043, 21120102036, 21361130020]
- National Basic Research Program of China (973 program) [2014CB239402]
- Natural Science Foundation of Liaoning Province [2014020010]
- Swedish Energy Agency
- K & A Wallenberg Foundation
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A highly active iron-based water-oxidation catalyst was electro-deposited from a CO2 saturated bicarbonate solution containing Fe2+. This catalyst (Fe-Ci) produces a current density of 10 mA cm(-2) at an overpotential of 560 mV and the activity remains constant over 18 h in the environmentally benign HCO3-/CO32- buffer (pH 9.75). A Tafel slope of 34 mV dec(-1) was obtained for Fe-Ci, which is lower than other reported values for iron-based catalysts.
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