Journal
CHEMICAL COMMUNICATIONS
Volume 52, Issue 24, Pages 4454-4457Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6cc00573j
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Funding
- National Key Technology Support Program of China [2015BAC04B01]
- National Natural Science Foundation of China [91334203, 21376074, 21321064]
- 111 Project of Ministry of Education of China [B08021]
- U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division
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We present a rational design and synthesis of a novel porous pyridine-functionalized polycarbazole for efficient CO2 capture based on the density functional theory calculations. The task-specific polymer, generated through a one-step FeCl3-catalyzed oxidative coupling reaction, exhibits a superior CO2 uptake at 1.0 bar and 273 K (5.57 mmol g(-1)).
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