Journal
CHEMICAL COMMUNICATIONS
Volume 52, Issue 59, Pages 9212-9215Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6cc04013f
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Funding
- Spanish Government [MAT2013-46753-C2-1-P, CTQ2014-53486-R]
- FEDER
- Swiss National Science Foundation (SNSF) [200021_160174]
- Engineering and Physical Sciences Research Council [EP/M005178/1] Funding Source: researchfish
- EPSRC [EP/M005178/1] Funding Source: UKRI
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A microfluidic chip has been used to prepare fibres of a porous polymer with high structural order, setting a precedent for the generation of a wide variety of materials using this reagent mixing approach that provides unique materials not accessible easily through bulk processes. The reaction between 1,3,5-tris(4-aminophenyl)benzene and 1,3,5-benzenetricarbaldehyde in acetic acid under continuous microfluidic flow conditions leads to the formation of a highly crystalline and porous covalent organic framework (hereafter denoted as MF-COF-1), consisting of fibrillar micro-structures, which have mechanical stability that allows for direct drawing of objects on a surface.
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