Journal
ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
Volume 27, Issue 19, Pages 23695-23706Publisher
SPRINGER HEIDELBERG
DOI: 10.1007/s11356-020-08785-2
Keywords
Selective catalytic oxidation; Cordierite; Catalyst; Denitration; Solid waste recycling; Resource utilization
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Funding
- National Natural Science Foundation of China [51704230, 41907255]
- Key Laboratory of Coal Resources Exploration and Comprehensive Utilization, Ministry of Natural Resources in P.R. China [KF2019-7]
- Shannxi Key Research and Development Project [2019ZDLSF05-05-01]
- 2019 Shaanxi Provincial Natural Science Basic Research Program Enterprise Joint Fund Project [2019JL-01]
- Natural Science Basic Research Plan in Shaanxi Province of China [2018JM5048]
- Xi'an Science and Technology Plan Project [2019217714GXRC013CG014-GXYD13.4]
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Low-value solid waste cordierite honeycomb ceramics were used as carrier of SCO denitration catalyst, and the active component was supported by the impregnation method to improve the performance of the catalyst. Firstly, the effect of calcination conditions on the denitration performance of the Mn-loaded cordierite catalyst was studied for the cordierite-loaded active component MnOX. Secondly, the preferred catalyst was reloaded with another active component to further improve its denitration performance; the bimetal ratios were affected by the denitration performance, which was, finally, characterized by XRD, XPS, and SEM. The result shows the following: (1) Mn-loaded cordierite prepared at 450 degrees C for 3 h has a good denitration effect; (2) the MnOX-CuOX/CR catalyst is superior to MnOX-FeOX/CR, MnOX-CoOX/CR, and MnOX-CeOX/CR; (3) the MnO2 crystal form in the single metal-supported catalyst plays a major role, and Cu2Mn3O8 in the bimetallic catalyst affects the performance and activity of the catalyst.
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