Journal
CHINESE JOURNAL OF CHEMISTRY
Volume 38, Issue 8, Pages 842-846Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cjoc.202000004
Keywords
Hexamethylenetetramine; Aryl aldehydes; Hydrogen; Amination; N; N-Dimethyl arylmethylamines
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Funding
- Beijing Municipal Science & Technology Commision [Z191100007219009]
- Chinese Academy of Science [GYZDY-SSW-SLH013]
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The Summary of main observation and conclusion Developing simple and green routes to access valuable chemicals is of significance. Herein, we present a green and novel route to synthesize N,N-dimethyl arylmethylamines (DAMAs) from hexamethylenetetramine (HMTA) and aryl aldehydes in the presence of hydrogen, and a series of DAMAs can be obtained in good yields. This approach opens the precedent for HMTA as N,N-dimethylamine source to synthesize chemicals with N,N-dimethylamine group, which has promising applications for N-containing chemicals synthesis.
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