Journal
CATALYSIS LETTERS
Volume 146, Issue 12, Pages 2417-2424Publisher
SPRINGER
DOI: 10.1007/s10562-016-1875-6
Keywords
Rhodium; Cobalt; Manganese; CNT growth catalyst; Higher alcohol synthesis; Carbon nanotubes; Nitrogen doping; Nanoparticles
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Funding
- Max Planck Society
- Federal Ministry of Education and Research (BMBF) [FKZ 03X0204C]
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Rh nanoparticles supported on commercial non-purified N-doped CNTs (NCNTs) containing residual CNT growth catalyst have been studied in hydrogenation of CO to higher alcohols. It has been found that Co and Mn residues in NCNTs are not inert, but change the catalyst under reaction conditions and efficiently promote the catalyst resulting in both increasing activity and selectivity to C2+ alcohols with time on stream. [GRAPHICS] .
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