Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 59, Issue 33, Pages 13722-13733Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.202004796
Keywords
CO2 conversion; covalent organic frameworks; heterogeneous catalysis; metal-organic frameworks; molecular separation
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Funding
- National Science Foundation of China [21431004, 21620102001, 21875136, 91856204]
- National Key Basic Research Program of China [2016YFA0203400]
- Key Project of Basic Research of Shanghai [17JC1403100, 18JC1413200]
- Shanghai Rising-Star Program [19QA1404300]
- China postdoctoral science foundation [2019M661483]
- postdoctoral innovative talent support program [BX20190195]
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Many sophisticated chemical and physical properties of porous materials strongly rely on the presence of the metal ions within the structures. Whereas homogeneous distribution of metals is conveniently realized in metal-organic frameworks (MOFs), the limited stability potentially restricts their practical implementation. From that perspective, the development of metal-covalent organic frameworks (MCOFs) may address these shortcomings by incorporating active metal species atop highly stable COF backbones. This Minireview highlights examples of MCOFs that tackle important issues from their design, synthesis, characterization to cutting-edge applications.
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