Journal
CARBON
Volume 100, Issue -, Pages 632-640Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.carbon.2016.01.018
Keywords
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Funding
- CSIR, New Delhi
- Department of Science and Technology (DST), New Delhi [GAP 3122]
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A novel graphene oxide (GO)-immobilized heteroleptic iridium complex was synthesized and demonstrated as a first heterogenized homogeneous catalyst for the production of dimethylformamide (DMF) from carbon dioxide, hydrogen, and dimethylamine. The synthesized hybrid catalyst showed comparable activity as homogeneous heteroleptic iridium complex with additional benefits such as facile recovery and recycling of the catalyst. After completion of the reaction, the heterogeneous catalyst was easily recovered by filtration, and reused for subsequent recycling processes without any significant change in the catalytic efficiency. (C) 2016 Elsevier Ltd. All rights reserved.
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