Journal
CHEMISTRYSELECT
Volume 5, Issue 8, Pages 2465-2468Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/slct.201904754
Keywords
Rhodium; C-H activation; Acylmethylation; Arylpurines; Sulfoxonium ylides
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Funding
- National Science Foundation of China [NSFC-21672035]
- Graduate Student Innovation Fund of Donghua University
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We have developed an efficient acylmethylation of C6 aryl- purines via C-H bond activation using the readily available sulfoxonium ylides as carbene precursors. The purine motif is the direction group. Our Rh-catalyzed acylmethylation offers excellent chemical yields and regioselectivity with good functional group tolerance.
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