4.7 Article

Tunable Curie temperature in layered ferromagnetic Cr5+xTe8 single crystals

Journal

APL MATERIALS
Volume 8, Issue 3, Pages -

Publisher

AMER INST PHYSICS
DOI: 10.1063/1.5143387

Keywords

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Funding

  1. National Key Research and Development Program of China [2018YFA0704300]
  2. National Natural Science Foundation of China [11804217]
  3. Program for Professor of Special Appointment (Eastern Scholar) at Shanghai Institutions of Higher Learning

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The relatively low Curie temperature (T-c) in recently discovered two-dimensional ferromagnetic (FM) materials has limited their potential applications in designing next generation electronics. Searching for new low-dimensional layered materials with room-temperature T-c is highly needed. Here, we report the study of layered FM materials Cr5+xTe8 (x = -0.10, 0.11, 0.56, 1) in which T-c can be well manipulated by the Cr content. Single crystalline Cr5+xTe8 samples have been synthesized and characterized by energy dispersive x-ray spectroscopy, x-ray diffraction, and magnetization measurements. We have found that T-c increases monotonically with Cr content and reaches 313 K at x = 1. While the FM coupling is enhanced with an increase in the Cr content, the antiferromagnetic (AFM) phase at low temperatures is suppressed. Due to the competition of FM and AFM phases, a wasp-waist loop is observed on isothermal magnetization curves. A magnetic flip occurs by changing the temperature and magnetic field to overcome the flipping energy barrier. Our results indicate that the Cr5+xTe8 system serves as a promising platform to tune the 2D ferromagnetism in layered materials.

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