Journal
ADVANCED SCIENCE
Volume 7, Issue 5, Pages -Publisher
WILEY
DOI: 10.1002/advs.201903088
Keywords
interfaces; ionic conductivity; lithium batteries; solid composite electrolytes
Categories
Funding
- National Natural Science Foundation of China [51672156]
- Local Innovative Research Teams Project of Guangdong Pearl River Talents Program [2017BT01N111]
- Guangdong Province Technical Plan Project [2017B010119001, 2017B090907005]
- Shenzhen Technical Plan Project [JCYJ20180508152210821, JCYJ20170817161221958, JCYJ20170412170706047]
- Tianjin Research Institute for Development Strategy of China's Engineering Science and Technology
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Solid composite electrolytes (SCEs) that combine the advantages of solid polymer electrolytes (SPEs) and inorganic ceramic electrolytes (ICEs) present acceptable ionic conductivity, high mechanical strength, and favorable interfacial contact with electrodes, which greatly improve the electrochemical performance of all-solid-state batteries compared to single SPEs and ICEs. However, there are many challenges to overcome before the practical application of SCEs, including the low ionic conductivity less than 10(-3) S cm(-1) at ambient temperature, poor interfacial stability, and high interfacial resistance, which greatly restrict the room temperature performance. Herein, the advances of SCEs applied in all-solid-state lithium batteries are presented, including the Li ion migration mechanism of SCEs, the strategies to enhance the ionic conductivity of SCEs by various morphologies of ICEs, and construction methods of the low resistance and stable interfaces of SCEs with both cathode and anode. Finally, some typical applications of SCEs in lithium batteries are summarized and future development directions are prospected. This work presents how it is quite significant to further enhance the ionic conductivity of SCEs by developing the novel SPEs with the special morphology of ICEs for advanced all-solid-state lithium batteries.
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