4.8 Article

Multifunctional full-visible-spectrum optoelectronics based on a van der Waals heterostructure

Journal

NANO ENERGY
Volume 66, Issue -, Pages -

Publisher

ELSEVIER
DOI: 10.1016/j.nanoen.2019.104107

Keywords

Low-powered; Van der Waals heterostructure; ReSe2; Optoelectronic memory; Charge storage; Multi-functionality

Funding

  1. Taiwan Ministry of Science and Technology [MOST 107-2119-M-005-006, 105-2112-M-005-002-MY3]
  2. Elemental Strategy Initiative
  3. CREST, JST [JPMJCR15F3]

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Multifunctional devices are expected to allow development of low-cost, highly integrated, and energy-efficient electronics for the internet of things (IoT) era. Here, we demonstrate an all-two-dimensional ReSe2/h-BN/graphene heterostructure (ReSe2 HS) consisting of a vertically coupled ReSe2 field-effect transistor and charge storage component, which possesses multifunctional characteristics for use in electronics and optoelectronics. As an electrically controlled non-volatile memory (NVM), the ReSe2 HS delivers high-performance multilevel data storage with a readout on/off current ratio exceeding 10(5) and excellent durability (> 10(4) s) at an ultralow V-ds of 50 mV, which benefits to the development of power saving devices. The ReSe2 HS design and high-photoresponsivity ReSe2 channel also achieve an energy efficient optical NVM with full-visible-spectrum distinction. Besides, the ReSe2 HS displays unique ambipolarity to operate as either an inverter or frequency doubler. We further propose a power-free ReSe2 HS optical memory matrix to simplify imaging systems. The ReSe2 HS shows promise for use in light-programmable information storage systems and neuromorphic computation with low power consumption.

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