4.7 Article

Hierarchical Porous RGO/PEDOT/PANI Hybrid for Planar/Linear Supercapacitor with Outstanding Flexibility and Stability

Journal

NANO-MICRO LETTERS
Volume 12, Issue 1, Pages -

Publisher

SHANGHAI JIAO TONG UNIV PRESS
DOI: 10.1007/s40820-019-0342-5

Keywords

RGO/PEDOT/PANI; Hierarchical; Porous; Supercapacitor; High performance

Funding

  1. Natural Science Foundation of Shenzhen University [2017004]
  2. Shenzhen Science and Technology Research Grant [JCYJ20170818142354137]
  3. Natural Science Foundation of Guangdong Province [2018A030310420]
  4. Guangdong Research Center for Interfacial Engineering of Functional Materials
  5. National Natural Science Foundation of China [51773118, 51202150, 51272161]

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Many hybrid electrodes for supercapacitors (SCs) are a reckless combination without proper structural design that keeps them from fulfilling their potential. Herein, we design a reduced graphene oxide/poly(3,4-ethylene-dioxythiophene)/polyaniline (RGO/PEDOT/PANI) hybrid with hierarchical and porous structure for high-performance SCs, where components fully harness their advantages, forming an interconnected and conductive framework with substantial reactive sites.Thus, this hybrid achieves a high capacitance of 535 F g(-1) along with good rate capability and cyclability. The planar SC based on this hybrid deliver an energy density of 26.89 Wh kg(-1) at a power density of 800 W kg(-1). The linear SC developed via modifying a cotton yarn with the hybrid exhibits good flexibility and structural stability, which operates normally after arbitrary deformations. This work provides a beneficial reference for developing SCs.

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