Journal
ADVANCED ENERGY MATERIALS
Volume 10, Issue 10, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/aenm.201903922
Keywords
conductive atomic force microscopy; electronic transport behavior; ferroelectricity; ion migration; perovskite materials; perovskite solar cells
Categories
Funding
- National Key Research and Development Program of China [2016YFA0202701, 2018YFA0703503]
- Overseas Expertise Introduction Project for Discipline Innovation (111 project) [B14003]
- National Natural Science Foundation of China [51991340, 51722203, 51672026, 51527802, 51702014, 51902021]
- Postdoctoral Research Foundation of China [2019M650488]
- State Key Laboratory for Advanced Metals and Materials [2018Z-03, 2019Z-04]
- Fundamental Research Funds for the Central Universities [FRF-TP-18-042A1, FRF-AS-17-002, FRF-TP-19-005A2]
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Metal halide perovskite materials, benefiting from a combination of outstanding optoelectronic properties and low-cost solution-preparation processes, show tremendous potential for optoelectronics and photovoltaics. However, the nanoscale inhomogeneities of the electronic properties of perovskite materials cause a number of difficulties, such as recombination, stability, and hysteresis, all of which seriously restrict device performance. Scanning probe microscopy, as a high-resolution imaging technique, has been widely used to connect local properties and micro-area morphologies to overall device performance. Conductive atomic force microscopy (C-AFM) can realize a real-space visualization of topography coupled with optoelectronic properties on a microscopic scale and thereby is uniquely suited to probe the local effects of perovskite materials and devices. The fundamental principles, alternative operation modes, and development of C-AFM are comprehensively reviewed, and applications in perovskite solar cells (PSCs) for electronic transport behavior, ion migration and hysteresis, ferroelectric polarization, and facet orientation investigation are discussed. A comprehensive understanding and summary of up-to-date applications in PSCs is beneficial to further fully exploit the potential of such an emerging technique, so as to provide a novel and effective approach for perovskite materials analysis.
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