Journal
ORGANIC LETTERS
Volume 22, Issue 4, Pages 1480-1484Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.0c00061
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Funding
- National Natural Science Foundation of China [31972145]
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A simple imine-based covalent organic framework (COF) as heterogeneous ligand for Pd-II-promoted Hcck reaction is reported. Good regioselectivity for a wide range of electronically unbiased olefins is obtained (linear/branched >100:1 in most cases). Related tests and density functional theory calculations are used to explore the reason underlying the high selectivity. This research opens a route for COF as an intriguing platform to control regioselectivity catalysis.
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