Journal
MOLECULES
Volume 25, Issue 3, Pages -Publisher
MDPI
DOI: 10.3390/molecules25030508
Keywords
fluoroalkyl iodides; EDA; noncovalent interaction; fluoroalkylated alkenes; DMA
Funding
- National Natural Science Foundation of China [21702241, 81760624, 21762053]
- Programs of Guizhou Province [2017-1225, 2018-1427]
- Guizhou Provincial Science & Technology 125-Plan Major Project [2015-039]
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Here, we describe a mild, catalyst-free and operationally-simple strategy for the direct fluoroalkylation of olefins driven by the photochemical activity of an electron donor-acceptor (EDA) complex between DMA and fluoroalkyl iodides. The significant advantages of this photochemical transformation are high efficiency, excellent functional group tolerance, and synthetic simplicity, thus providing a facile route for further application in pharmaceuticals and life sciences.
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