Journal
MATERIALS TECHNOLOGY
Volume 35, Issue 9-10, Pages 594-599Publisher
TAYLOR & FRANCIS LTD
DOI: 10.1080/10667857.2020.1718845
Keywords
Potassium & xfeff;-ion batteries; anodedealloying; co(3)o(4); two-dimensional material
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Funding
- National Natural Science Foundation of China [51972198]
- State Key Program of National Natural Science of China [61633015]
- Project of the Taishan Scholar [ts201511004, tsqn201812002]
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Potassium has attracted enormous attention as the promising resourceful alternative to lithium for rechargeable batteries. However, the developing of high-energy electrode materials remains a key challenge for potassium-ion batteries (KIBs). Herein, 2D nanoporous cobaltosic oxide (Co3O4) is synthesised by scalable chemical dealloying methods from bulk Al-Co alloy. It is found that the morphology of Co3O4 can be controlled by adjusting the dealloying time. As anode materials for KIBs, the as prepared Co3O4 nanosheets delivered a reversible capacity of 417 mA h g(-1) at a constant current density of 89 mA g(-1) and a good capacity retention even after 300 cycles. The special 2D nanoporous structure is beneficial to buffer volume expansion and enhance ionic diffusion, which is accounted for the good electrochemical performance. The synthesis method and the special structure may be interesting for researchers in other fields such as supercapacitor, catalyst, and sensors.
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