Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 142, Issue 4, Pages 1686-1691Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.9b11328
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Funding
- ERATO program of the JST [JPMJER1302]
- CREST program of the JST [JPMJCR19R1]
- JSPS KAKENHI [19H05463, JP26810057, JP16H00907, JP17K1955, JP18H02019]
- JSPS Research Fellowship for Young Scientists [18J10996]
- Sumitomo Foundation [141495]
- DAIKO Foundation
- World Premier International Research Center Initiative (WPI), Japan
- Grants-in-Aid for Scientific Research [18J10996] Funding Source: KAKEN
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Graphene nanoribbons (GNRs), nanometer-wide strips of graphene, are attracting significant attention in materials science as candidates for next-generation carbon materials. As their physical properties mainly depend on their structures, the precise synthesis of structurally well-defined GNRs is highly desirable to control their properties. Herein, we report a step-growth annulative pi-extension polymerization that allows for the rapid and modular synthesis of cove-type GNRs with pyrene and/or coronene diimide repeating units. The structures and photophysical properties of the separated GNRs were confirmed by various spectroscopic analyses. In addition, gas-blow-assisted uniform on-surface self-assembly of the GNRs was accomplished.
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