Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 85, Issue 5, Pages 3942-3948Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.9b03205
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Funding
- National Natural Science Foundation of China [21602001, 21922109, 21672196, 21831007, 39837134]
- Nanjing Tech University [39837134]
- Fundamental Research Funds for the Central Universities of China [WK2060190086]
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An organocatalyzed aerobic benzylic C-H oxidation of alkyl and aryl heterocycles has been developed. This transition metal-free method is able to overcome the electron-withdrawing effect as well as product-inhibition effects in heterobenzylic radical oxidation. A variety of ketones bearing N-heterocyclic groups could be prepared under relatively mild conditions with moderate to high yields.
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