Journal
INTERNATIONAL JOURNAL OF MECHANICAL SCIENCES
Volume 177, Issue -, Pages -Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.ijmecsci.2020.105552
Keywords
Two-way shape memory polymer; Constitutive model; Reversible actuation; Semicrystalline polymer; Model sensitivity analysis
Categories
Funding
- National Science Foundation [1736136]
- NASA [NNX16AQ93A, NASA/LEQSF(2016-19)-Phase3-10]
- NASA [895000, NNX16AQ93A] Funding Source: Federal RePORTER
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Recently, two-way shape memory effect (2W-SME) has been demonstrated in several types of shape memory polymers (SMPs). Unlike classical one-way shape memory effect (1W-SME), these polymers can switch back and forth repeatedly between two different shapes without subsequent programming procedure. The reversible actuation can be realized either under a constant external tensile load, which is referred to as quasi 2W-SME, or under zero load, which is referred to as true 2W-SME. Most recently, actuation under an external compressive load, which is referred to as advanced 2W-SME, has also been discovered. Test results have shown that semicrystalline 2W-SMPs exhibit 2W-SME in two distinct regions due to two different mechanisms: one is due to entropic elasticity above the crystallization temperature, and the other is due to melt/crystallization transition below the crystallization temperature. While several constitutive models have been developed over the years for semicrystalline 2W-SMPs, there is currently a lack of effort towards modeling the true and advanced 2W-SME within the two-mechanism framework. In this study, we developed a thermomechanical constitutive model which captured both the entropic elasticity and melt/crystallization events. The modeling results and test results show reasonable agreement. It is found that the model captured the three types of 2W-SMEs: quasi 2W-SME, true 2W-SME, and advanced 2W-SME. It is also found that proper tensile programming before the first thermomechanical cycle can make a semicrystalline SMP exhibit all the three types of 2W-SMEs. This study may serve as a design tool to enhance applications of semicrystalline 2W-SMPs in engineering structures and devices.
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