Journal
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
Volume 59, Issue 1, Pages 154-165Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.iecr.9b04416
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Funding
- National Natural Science Foundation of China [51703137]
- Fundamental Research Funds for the Central Universities of China [2015SCU11008]
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Electromagnetic interference (EMI) shielding materials, entailing the efficient electromagnetic (EM) shielding and high EM wave (EMW) absorption, have become a further requirement for the upcoming 5G communication. Herein, the composite films with a multilayer sandwich structure from cellulose solution in ferric metal- organic frameworks (MOFs) (MIL-88B)-derived magnetic carbon-based materials (C-MIL-88B) and graphene nanoplates (GNPs) are successfully fabricated through a filtration-assisted self-assembly method. The resultant C-MIL-88B/GNP films possess satisfactory saturation magnetization and considerable conductivity with the introduction of Fe3O4-C. Interestingly, the composite film with five layers (0.12 mm) obtains a reliable EMI shielding effectiveness of 28 dB in the X-band frequency range, while the power coefficient of absorption (A) is up to 86%. The improved microwave absorption and attenuation properties of the C-MIL-88B/GNP film are resulted from the synergistic effect of dielectric loss, magnetic loss, and multilayer structure. This work highlights the potential of MOFs/GNP composite films in absorption-dominated EMW protection fields.
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