Journal
FUEL
Volume 264, Issue -, Pages -Publisher
ELSEVIER SCI LTD
DOI: 10.1016/j.fuel.2019.116616
Keywords
CO2 capture; Absorption; Amine; CO2 solubility; Modeling
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In absorptive removal of CO2 by aqueous alkanolamine solvent, as the most prevalent CO2 capture technique, equilibrium absorption capacity of CO2 is a significant parameter for assessing the efficiency of absorption systems. In this study, unique computational models are presented to estimate CO2 solubility in commonly used amines. A series of models, including genetic algorithm-adaptive neuro fuzzy inference system (GA-ANFIS), particle swarm optimization ANFIS (PSO-ANFIS), coupled simulated annealing-least squares support vector machine (CSA-LSSVM) and radial basis function (RBF) neural networks were developed to estimate CO2 equilibrium absorption capacity in twelve aqueous amine solutions. The model inputs comprise of CO2 partial pressure, temperature, amine concentration in aqueous solution, molecular weight, hydrogen bond donor/acceptor count, rotatable bond count and complexity of the amines. The obtained results affirm that among proposed models, LSSVM exhibits more promising results with an excellent compatibility with experimental values. In detail, both mean square errors and average regression coefficient (R-2) of LSSVM model are 0.02 and 0.9338, respectively. Moreover, it is confirmed that the proposed LSSVM model has better accuracy compared to the other models.
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