Journal
ENVIRONMENTAL POLLUTION
Volume 258, Issue -, Pages -Publisher
ELSEVIER SCI LTD
DOI: 10.1016/j.envpol.2019.113825
Keywords
Gamma spectrometry; Radiological parameters; Uranium; Radium; Thorium; Soil pollution; Mining; Uranium decay chain
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The establishment of a screening index would be a powerful tool to decide whether abandoned uranium mining areas should be rehabilitated or decommissioned. Thus, in this work we established a radiological index which uses the activity concentrations of different groups of gamma emitters from the natural radioactive series of U-238, U-235, and Th-232, as well as K-40 and Cs-137. These activity concentrations were calculated by using the absorbed gamma radiation dose value of 175 nGy h(-1) specified in the U.S. Code of Federal Regulations. We studied our index in an abandoned uranium mining area in Salamanca, Western Spain, and found that the most influential factors in this area were the presence of organic matter in the soil and the possible effect that plants and fungi may have on the retention of these aforementioned radionuclides. In addition, the results showed that contaminants are migrating in an easterly direction in line with the prevailing wind direction and we were able to identify areas in which the radiological risk is likely high. The mean effective dose rate was 2.51 +/- 0.98 mSv y(-1) which was equivalent to the levels obtained in previous works. (C) 2019 Elsevier Ltd. All rights reserved.
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