Journal
CHEMSUSCHEM
Volume 13, Issue 6, Pages 1392-1408Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cssc.201902688
Keywords
electrochemistry; molybdenum; sulfur; supported catalysts; surface chemistry
Funding
- Natural Science Fund of China [11722543]
- National Key Research and Development Program of China [2017YFA0206703]
- Fundamental Research Funds for the Central Universities [WK2060190074, WK2310000066]
- Anhui Provincial Natural Science Foundation [1808085QB35]
- Science and Technology Program of Taizhou [14GY03]
- Excellent Young Scientist Fund of Taizhou University [2017JQ004]
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Two-dimensional molybdenum disulfide (MoS2) nanosheets attract great interest for applications in lithium-sulfur (Li-S) batteries, due to their unique physical and chemical properties, which originate from diverse chemical compositions and unique electronic structures. In recent years, many efforts have been devoted to employing MoS2 as a polysulfide immobilizer and catalyst, functional separator, and Li-metal protection for Li-S batteries through structural design and electronic modulation. A fundamental understanding of the interplay between structural features, electronic properties, and advanced electrochemical performance is crucial for providing valuable insights for the development of Li-S batteries. In this regard, recent advances in Li-S batteries with 2D MoS2 materials are summarized from the perspective of structural design and electronic modulation. Finally, future prospects and remaining challenges of MoS2 for Li-S batteries are highlighted.
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