Journal
CHEMOSPHERE
Volume 239, Issue -, Pages -Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.chemosphere.2019.124701
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Funding
- National Institute of Environmental Health Sciences
- US Environmental Protection Agency [NIEHS P01 ES11261, R01 ES014575, R01 ES020349, R01 ES024381, R01 ES025214, R01 ES027224, R01 ES028277, P30 ES006096, EPA P01 R829389]
- University of Cincinnati [2T32GM063483-1]
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Polybrominated diphenyl ethers, a class of flame retardants and endocrine disruptors, have been substituted in new products by organophosphate (OPFR) and replacement brominated flame retardants (RBFR). OPFRs and RBFRs readily migrate from consumer products into dust where humans are exposed via incidental ingestion and inhalation. We quantified concentrations and loadings of OPFRs and RBFRs in house dust samples (n = 317) collected from the homes of Cincinnati women between 2003 and 2006 and examined their associations with demographic and house characteristics. Tris-(1-chloro-2-propyl)-phosphate (TCIPP, geometric mean [GM]: 2140 ng g(-1), range: 70.1-166,000 ng g(-1)), tris-(1,3-dichloro-2-propyl)-phosphate (TDCIPP, GM: 1840 ng g(-1), range: 55.2-228,000 ng g(-1)), triphenyl phosphate (TPHP, GM: 1070 ng g(-1), range: 34.1-62,100 ng g(-1)), 2-ethylhexyl-2,3,4,5-tetrabromobenzoate (EH-TBB, GM: 59.5 ng g(-1), range: 2.82-7800 ng g(-1)), and bis-(2-ethylhexyl)-tetrabromophthalate (BEH-TEBP, GM: 121 ng g(-1), range 2.17-13,600 ng g(-1)) were all detected in >90% of dust samples; tris-(2-chloroethyl)phosphate (TCEP, GM: 669 ng g(-1), range: 56.8-160,000 ng g(-1)) was detected in 80.1% of samples. Concentrations of EH-TBB and BEH-TEBP increased in house dust from 2003 to 2006. The number of people living in the home, race, education, floor type, and year of sample collection were associated with some OPFR and RBFR concentrations and loadings. This study suggests that OPFRs and RBFRs were ubiquitous in house dust during the PBDE phase-out and justifies more research on the consequences of exposure to these environmental chemicals. (C) 2019 Elsevier Ltd. All rights reserved.
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