Journal
CHEMISTRY-AN ASIAN JOURNAL
Volume 15, Issue 7, Pages 1132-1139Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/asia.202000001
Keywords
CO2 activation; Metal-organic framework; Nanocrystalline Zeolite; Integrated Porous Framework; Insertion Reactions
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Funding
- Director's Fellowship Funding Source: Medline
- DST-SERB, New Delhi [EMR/2016/001408] Funding Source: Medline
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The conversion of CO2 to useful chemicals, especially to atom economical products, is the best approach to utilize an excess of CO2 present in the atmosphere. In this study, a metal-organic framework (ZIF-8) is integrated with nanocrystalline zirconosilicate zeolite to develop an integrated porous catalyst for CO2 insertion reactions. The catalyst exhibits excellent activity for the CO2 insertion reaction of epoxide to produce cyclic carbonate in neat condition without the addition of any co-catalyst. The catalyst is stable and recyclable during the cyclic carbonate synthesis. Further, the catalyst also exhibits very good activity in another CO2 insertion reaction to produce quinazoline-2,4(1H, 3H)-dione.
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