Journal
CHEMICAL ENGINEERING JOURNAL
Volume 380, Issue -, Pages -Publisher
ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2019.122475
Keywords
Polymeric film; MXene; Multilayered structure; Electromagnetic interference shielding; Thermal conductivity; Flame retardancy
Categories
Funding
- China Postdoctoral Science Foundation [2018M642780]
- Opening Project of State Key Laboratory of Polymer Materials Engineering (Sichuan University) [sklpme2019-4-31]
- Startup Research Fund of Zhengzhou University [32211146]
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With the miniaturized and high-frequency development in electronic products, polymeric films synchronously with high electromagnetic interference (EMI) shielding effectiveness (SE) and thermal conductivity (TC) are urgently needed. In this work, poly (vinyl alcohol)/transition metal carbide (PVA/MXene) films featured with alternating multilayered structure were fabricated through multilayered casting. The continuous MXene layer provided a compact network for conducing heat and electron, endowing the multilayered film with excellent EMI SE and TC synchronously. In particular, the 27-mu m-thick PVA/MXene multilayered film (containing 19.5 wt % MXene in total) exhibited an electrical conductivity of 716 S/m, a maximum EMI SE of 44.4 dB and a specific EMI SE (SSEt) of 9343 dB cm(2) g(-1). Meanwhile, the multilayered film showed a high in-plane TC of 4.57 W/mK, enhanced by almost 23-fold compared with that of neat PVA. Moreover, the multilayered architecture endowed the film with remarkable anti-dripping performance. This work provides a novel and feasible strategy for fabricating flame-retardant polymeric thermal conducive and EMI shielding films, which will have enormous prospect in advanced electrical devices.
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