Journal
APPLIED SURFACE SCIENCE
Volume 504, Issue -, Pages -Publisher
ELSEVIER
DOI: 10.1016/j.apsusc.2019.144487
Keywords
Laser-induced graphene; Gelatin; Morphology transition; Co3O4; Supercapacitor
Categories
Funding
- National Natural Science Foundation of China [51775197]
- Science and Technology Planning Project of Guangdong Province [2018A050506007]
- Guangzhou Science and Technology Program Project [201704020090]
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Recent trends have witnessed laser induced graphene (LIG) syntheses on various materials from synthetic polymers to natural precursors. Herein, porcine skin derived gelatin was used as a medium to modify the surface morphology and nanoparticle distribution of in situ synthesized Co3O4 /LIG on polyimide (PI) film. By varying the applied laser fluence, the surface morphology of LIG transitions from a 3D porous structure to a multilayered structure, Co3O4 progressively distributes from the surface to the inside of the LIG structure, and the structure changes from a sphere to a whisker-like shape. These altered attributes contribute to distinct differences in the double layer capacitance and pseudocapacitance behaviors of Co3O4 /LIG, as reflected in its associated electrochemical performance. Additionally, a facile fabrication strategy including simple casting and peeling steps was used to generate stretchable microsupercapacitors (MSCs) on a waterborne polyurethane (WPU) substrate. The as-prepared stretchable MSCs present outstanding areal capacitance and excellent mechanical flexibility, whereas their electrochemical differences are significantly minimized and dominated by their inner structures.
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