Journal
APPLIED SURFACE SCIENCE
Volume 501, Issue -, Pages -Publisher
ELSEVIER
DOI: 10.1016/j.apsusc.2019.144245
Keywords
g-C3N4; P-S co-doping; Ag deposition; Photocatalytic inactivation
Categories
Funding
- National Natural Science Foundation of China [21406094]
- Doctoral Innovation Program of Affiliated Hospital of Jiangsu University [JDFYRC2017002]
- College Natural Science Research Program of Jiangsu Province, China [13KJB350001]
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Photocatalytic inactivation has been proved to be an effective strategy for controlling biohazards. Herein, the novel Ag deposited phosphorus and sulfur co-doped g-C3N4 (PSCN) composites with different Ag content were constructed via a facile calcination combining with biogenic-reduction method for inactivating Escherichia coli (E. coli). The detailed characterization results indicated that P and S elements were successfully co-doped into g-C3N4 (CN) lattice and Ag nanoparticles (NPs) were evenly deposited on the surface of PSCN with diameter range of 4-20 nm. The Ag/PSCN at depositing amount of 4 wt% (Ag/PSCN-4) achieved the strongest photocatalytic inactivation along with excellent stability, which could completely inactivate 7.0 log cells of E. coli within 60 min of visible light irradiation. This improved bactericidal performance was mainly attributed to the synergistic effects of P-S co-doped together with Ag deposition, which resulted in the increased visible light utilization, the improved separation and transfer efficiency of photo-induced charge carriers. Moreover, active species trapping experiments revealed that the generated superoxide radicals (O-center dot(2)-) and holes (h(+)) played the significant roles in photocatalytic inactivation process. Our present work presented a promising and environmentally friendly strategy to enhance the photocatalytic capacities of CN based composites for pathogens inactivation.
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