4.8 Review

Performance-Enhancing Approaches for PEDOT:PSS-Si Hybrid Solar Cells

Journal

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 60, Issue 10, Pages 5036-5055

Publisher

WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201910629

Keywords

heterojunctions; hybrid solar cells; nanostructures; PEDOT; PSS; silicon

Funding

  1. National Research Foundation of Korea (NRF) - Korea government (MSIP) [2018R1A2A1A05077194]
  2. Center for Advanced Soft-Electronics - Ministry of Science and ICT [2012M3A6A5055225]
  3. Wearable platform Materials Technology Center - Ministry of Science, ICT and future Planning [2016R1A5A1009926]
  4. Ulsan City of UNIST (Ulsan National Institute of Science Technology) [1.200042]
  5. National Natural Science Foundation of China [51702032, 61504015, 62074022]
  6. Natural Science Foundation of Chongqing [cstc2017jcyjA0752, cstc2018jszx-cyzd0603, cstc2018jcyjAX0375, cstc2018jcyjAX0556, cstc2017rgznzdyfX0030, cstc2017jcyjAX0451, cstc2017rgznzdyfX0023, cstc2020jcyj-msxmX0851]
  7. Key Laboratory of Low-grade Energy Utilization Technologies and Systems [LLEUTS-2017004, LLEUTS-2019001]
  8. Venture & Innovation Support Program for Chongqing Overseas Returnees [cx2019107]
  9. Fundamental Research Funds for the Central Universities [2019CDXYDL0007, 2020CDJ-LHZZ-044, 2020CDJQY-A055, 2018CDQYDL0051]
  10. Institute of Civil Military Technology Cooperation Center (ICMTC) - Defense Acquisition Program Administration
  11. Ministry of Trade, Industry and Energy
  12. Defense Acquisition Program Administration of Korea [18-CM-SS-13]
  13. Agency for Defense Development (ADD), Republic of Korea [18-CM-SS-13] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)

Ask authors/readers for more resources

The emerging energy crisis has drawn global attention to solar cells, particularly hybrid solar cells like organic-Si HSCs. Among them, PEDOT:PSS/Si HSCs show promising efficiency improvements through methods such as PEDOT:PSS modification and interface layer optimization.
The emerging energy crisis has focused significant worldwide attention on solar cells. Although crystalline silicon solar cells are currently widely used, their high cost limits the development of solar power generation. Consequently, hybrid solar cells are becoming increasingly important, especially organic-Si hybrid solar cells (HSCs). Organic-Si HSCs combine a mature technology and high efficiency with the low-temperature manufacturing process and tunable optoelectronic properties of organic solar cells. The organic material can be P3HT, carbon nanotubes, graphene, and PEDOT:PSS. Here we review the performance of PEDOT:PSS/Si HSCs and methods for improving their efficiency, such as PEDOT:PSS modification, optimization of the trapping effect, passivation of the silicon surface, addition of an interface layer, improvement of a back contact, and optimization of the metal top electrode. This Review should help fill the gap in this area and provide perspectives for the future development of the PEDOT:PSS/Si HSCs.

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