Journal
ACS OMEGA
Volume 4, Issue 21, Pages 19106-19115Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsomega.9b02322
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Funding
- Natural Sciences and Engineering Research Council of Canada
- University of Western Ontario
- Government of Canada
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A novel bioorthogonal gold nanoparticle (AuNP) template displaying interfacial nitrone functional groups for bioorthogonal interfacial strain-promoted alkyne-nitrone cycloaddition reactions has been synthesized. These nitrone-AuNPs were characterized in detail using H-1 nuclear magnetic resonance spectroscopy, transmission electron microscopy, thermogravimetric analysis, and X-ray photoelectron spectroscopy, and a nanoparticle raw formula was calculated. The ability to control the conjugation of molecules of interest at the molecular level onto the nitrone-AuNP template allowed us to create a novel methodology for the synthesis of AuNP-based radiolabeled probes.
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