Journal
ACS ENERGY LETTERS
Volume 4, Issue 12, Pages 2960-2974Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsenergylett.9b02063
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Funding
- European Union H2020 Programme under a European Research council Consolidator grant [MOLEMAT] [726360]
- Spanish ministry of Science and Technology [RTI2018-102292-B-I00]
- National Natural Science Foundation of China Major International (Regional) Joint Research Project [51661135023, 51961165106]
- National Natural Science Foundation of China [21673091, 21975088]
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Three-dimensional halide-based perovskites have emerged as promising semiconducting light harvesters for thin-film solar cell fabrication; however, their intrinsic instability under humidity restricts their potential commercialization. To address such challenges, the development of low-dimensional/layered Dion-Jacobson (DJ) phase perovskites has recently gained substantial attention due to their intriguing environmental stability and competitive power conversion efficiency. In this Review, we have screened and focused our investigation on the DJ phase in layered perovskites for solar cell fabrication, especially elucidation of the active role played by organic spacer cations. We also discuss the possible strategies that can be employed to further push the performance of DJ-based perovskite solar cells.
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