Journal
SENSORS AND ACTUATORS B-CHEMICAL
Volume 297, Issue -, Pages -Publisher
ELSEVIER SCIENCE SA
DOI: 10.1016/j.snb.2019.126753
Keywords
Landfill gas emissions; Quartz-enhanced photoacoustic spectroscopy; Optical gas sensor; Gas V-T relaxation; Combined vibration of quartz tuning fork
Funding
- National Key Research and Development Program of China [2017YFA0304203]
- National Natural Science Foundation of China [61622503, 61805132, 61575113, 11434007]
- Scientific Research Foundation [227545028]
- Changjiang Scholars and Innovative Research Team in University of Ministry of Education of China [IRT_17R70]
- 111 project [D18001]
- Outstanding Innovative Teams of Higher Learning Institutions of Shanxi
- Shanxi 1331 Project key subjects construction
- Applied basic research program of Shanxi province [201801D221174]
- THORLABS GmbH
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A quartz-enhanced photoacoustic spectroscopy methane (CH4) sensor with vibrational to translational (V-T) relaxation self-calibration was realized and tested for atmospheric CH4 detection near a landfill. To normalize the influence of H2O vapor on the CH4 energy relaxation rate, CH4 and H2O concentrations were detected simultaneously by means of a frequency division multiplexing technique, in which a custom quartz tuning fork was operated in the fundamental and first overtone combined vibration mode. A continuous wave, thermo-electrically cooled distributed feedback interband cascade laser emitting at 3.3 mu m and a near-infrared DFB laser emitting at 1.37 mu m were used as the excitation source for CH4 and H2O detection, respectively. A theoretical model of V-T relaxation and self-calibration method were developed to allow this CH4 sensor to have a simple setup and a small sensor size. Continuous field measurements were carried out near the largest sanitary landfill in Shanxi province, China, to demonstrate the stability and ruggedness of the realized CH4 sensor.
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