Journal
REACTIVE & FUNCTIONAL POLYMERS
Volume 143, Issue -, Pages -Publisher
ELSEVIER
DOI: 10.1016/j.reactfunctpolym.2019.104340
Keywords
Porphyrin; Benzobisoxazole; Linear polymer; Photocatalyst; Rhodamine B
Funding
- Science and Technology Innovation Fund of Changchun University of Science and Technology [XJJLG-2016-05, XJJLG-2017-07]
- Research Foundation of Education Department of Jilin Province [JJKH20190582KJ]
- Research Foundation of Science & Technology Department of Jilin Province [20190303069SF]
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In this study, a novel 1D porphyrin-based polymer, polyphenylporphyrin benzobisoxazole, namely P(PPor-BBO), was synthesized via polycondensation between 5, 15-bis(4-carboxyphenyl)-10, 20-diphenylporphyrin and 4,6-diaminoresor-cinol dihydrochloride. The P(PPor-BBO) is a 1D fully-conjugated heterocyclic aromatic polymer with co-linear and co-planar rigid backbone. Extended fully pi-conjugated systems not only enhance chemical stability and lead to insolubility, but also improve photocatalytic active units and light-harvesting capability in the visible-light region. As a result, P(PPor-BBO) shows excellent photocatalytic performance for rhodamine B degradation (150 min, 98%) under visible-light irradiation. It also exhibits easy recyclability and sustainability, indicating it could be as environmentally-friendly catalyst for organic dye wastewater treatment.
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