Journal
ORGANIC LETTERS
Volume 21, Issue 23, Pages 9311-9314Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.9b03342
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Funding
- Japan Society for the Promotion of Science (JSPS) [JP18H02051, JP17K19164, 19K22191, JP18K14228]
- Mitsubishi Foundation
- Iketani Science and Technology Foundation
- Hyogo Science and Technology Association
- Kinoshita Memorial Enterprise
- Grants-in-Aid for Scientific Research [19K22191] Funding Source: KAKEN
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Efficient thermally activated delayed fluorescence materials based on the multiple resonance effect were synthesized by nucleophilic substitution and electrophilic C-H borylation, featuring a small energy gap between the singlet and triplet state, high photoluminescence quantum yield, and narrow emission band. Organic light-emitting diodes employing these materials as emitters exhibited sky-blue emission with a high external quantum efficiency of 21.4% and a narrow full width at half-maximum of 33 nm.
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