Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 141, Issue 45, Pages 18004-18008Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.9b10625
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Funding
- National Natural Science Foundation of China [21632004, 21871120]
- Natural Science Foundation of Gansu Province [18JR4RA003]
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Methodology development of robust link-ages is fundamentally important for the synthesis and application of covalent organic frameworks (COFs). We report herein a new strategy based on multicomponent reactions (MCRs) to construct ultrastable COFs. With the one-pot formation of five covalent bonds in each cyclic joint, a series of imidazole-linked COFs were robustly constructed through the Debus-Radziszewski MCR from three easily available components. By reaching a higher level of complexity and precision in covalent assembly, this research explores a new direction in integrating sophisticated reversible/irreversible reactions to construct crystalline porous frameworks.
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