Journal
JOURNAL OF PHYSICAL CHEMISTRY C
Volume 123, Issue 45, Pages 27363-27368Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.jpcc.9b08101
Keywords
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Funding
- National Natural Science Foundation of China [51602023]
- State Key Laboratory of New Ceramic and Fine Processing, Tsinghua University [KF201816]
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A series of WS2-MoS2 composites with different phase ratios have been successfully constructed. First, WS2 with hexagonal phase structure has been achieved by directly annealing a mixture of commercial W and S powders in an Ar atmosphere. Then the hydrothermal method is utilized to realize the epitaxial growth of MoS2 onto the surface of WS2. The dual-petal nanostructure of WS2-MoS2 composites has been revealed by scanning electron microscopy and transmission electron microscopy. The measurement of the optoelectronic property illustrates that WS2-MoS2 heterostructures can present more active sites and a higher effective separation of carriers than can bare WS2 and MoS2. Specifically speaking, 4WS(2)-96MoS(2) can cause the complete degradation of methylene blue within 150 min, and the difference value of the photocurrent can reach a value of 26 mu A, which obviously outperforms that of bare MoS2 and WS2. These aforementioned improved performances are closely related to this rationally designed structure for WS2-MoS2 heterostructures and are expected to be promising applications in the field of optoelectronic devices.
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