Journal
INORGANIC CHEMISTRY
Volume 58, Issue 22, Pages 15029-15033Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.inorgchem.9b02481
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Funding
- NSFC [51872297, 51890864]
- Fujian Institute of Innovation [FJCXY18010201]
- Youth Innovation Promotion Association in CAS
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In the military and civilian fields, with the development of new technologies, high-powered nonlinear optical (NLO) crystals demonstrate broad application prospects. In this work, for purposes of designing a better NLO material, a new chalcogenide Rb10Zn4Sn4S17 was successfully designed with a high temperature solid-state method on the basis of previously reported compound Sr3MnSn2S8. The experimental results indicate that Rb10Zn4Sn4S17 possesses a prominent band gap of 3.59 eV, compared with the laser damage threshold (LDT) of Sr3MnSn2S8 (3 times that of AgGaS2); Rb10Zn4Sn4S17 shows an outstanding LDT about 5 times that of AgGaS2. Meanwhile, it has an ideal second harmonic generation (SHG) response approximately 0.7 times that of AgGaS2.
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