Journal
HELVETICA CHIMICA ACTA
Volume 102, Issue 12, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/hlca.201900223
Keywords
enantioselectivity; chiral Lewis acids; radical reactions; conjugate additions; cyclic ketones
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Funding
- NIH [NIH-GM-54656]
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Enantioselective conjugate radical addition to 2-acyloxymethyl cycloalkenones proceeds in high yield with outstanding diastereoselectivity and excellent enantioselectivity using chiral salen Lewis acids. The process provides access to 2,3-disubstituted cycloalkanones, a structural motif present in natural products.
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