Journal
CHINESE JOURNAL OF CHEMISTRY
Volume 37, Issue 12, Pages 1229-1233Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cjoc.201900296
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Funding
- National Natural Science Foundation of China [21772202, 21701073, 21831008]
- Beijing Municipal Science & Technology Commission [Z181100004218004]
- Beijing National Laboratory for Molecular Sciences [BNLMS-CXXM-201901]
- Fundamental Research Funds for the Central Universities [lzujbky-2017-12, lzujbky-2019-kb06]
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of main observation and conclusion Herein, unprecedented rhenium-catalyzed decarboxylative oxytri-/difluoromethylation and Heck-type trifluoromethylation of styrenes have been developed by using hypervalent iodine(III) reagents derived from cheap, stable, and easy-handling fluorinated carboxylic acids. Mechanistic studies revealed a radical decarboxylative trifluoromethylation pathway occurring in these reactions.
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