Journal
CHEMISTRY-AN ASIAN JOURNAL
Volume 15, Issue 15, Pages 2364-2370Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/asia.201901433
Keywords
CO2 capture; mixed matrix membranes; MXene; Pebax; transport channels
Categories
Funding
- National Natural Science Foundation of China [51861135203, 21490585, 21776125, 21922805]
- Innovative Research Team Program by the Ministry of Education of China [IRT_17R54]
- Topnotch Academic Programs Project of Jiangsu Higher Education Institutions (TAPP)
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Mixed matrix membranes (MMMs) made from inorganic fillers and polymers is a kind of promising candidate for gas separation. In this work, two-dimensional MXene nanosheets were synthesized and incorporated into a polyether-polyamide block copolymer (Pebax) matrix to fabricate MMM for CO2 capture. The physicochemical properties of MXene nanosheets and MXene/Pebax membranes were studied systematically. The introduction of MXene nanosheets provided additional molecular transport channels and meanwhile enhanced the CO2 adsorption capacity, thereby enhancing both the CO2 peremance and CO2/N-2 selectivity of Pebax membrane. The optimized MXene/Pebax membrane with a MXene loading of 0.15 wt % displayed a high separation performance with a CO2 permeance of 21.6 GPU and a CO2/N-2 selectivity of 72.5, showing potential application in CO2 capture.
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