Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 59, Issue 3, Pages 1113-1117Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201911529
Keywords
nitrogen doping; polycyclic aromatic hydrocarbons; pyrene-fused azaacenes; singlet fission; tetracene
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Funding
- Basque Science Foundation for Science (Ikerbasque)
- POLY-MAT
- University of the Basque Country (Grupo de Investigacin) [GIU17/054]
- University of the Basque Country (SGIker)
- Gobierno Vasco (BERC program)
- Gobierno de EspaCa (Ministerio de Economa y Competitividad) [CTQ2016-77970-R]
- European Research Council (ERC) under the European Unions Horizon 2020 research and innovation programme [722951]
- Emerging Fields Initiative (EFI) Singlet Fission - FAU
- Cluster of Excellence Engineering of Advanced Materials (EAM)
- SolTech (Solar Technologies go Hybrid), an initiative of the Bavarian State Government
- Portuguese Foundation for Science and Technology (FCT) [PTDC/FIS-NAN/4662/2014, IF/00894/2015]
- CICECO-Aveiro Institute of Materials, FCT [UID/CTM/50011/2019]
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Singlet fission has emerged as a promising strategy to avoid the loss of extra energy through thermalization in solar cells. A family of dimers consisting of nitrogen-doped pyrene-fused acenes that undergo singlet fission with triplet quantum yields as high as 125 % are presented. They provide new perspectives for nitrogenated polycyclic aromatic hydrocarbons and for the design of new materials for singlet fission.
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