Journal
SCIENCE ADVANCES
Volume 5, Issue 8, Pages -Publisher
AMER ASSOC ADVANCEMENT SCIENCE
DOI: 10.1126/sciadv.aax0648
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Funding
- National Nature Science Foundation for Distinguished Young Scholars [21425417]
- National Natural Science Foundation of China [21835005, U1862109, 21704071]
- Priority Academic Program Development of Jiangsu Higher Education Institutions
- Postgraduate Research & Practice Innovation Program of Jiangsu Province
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Gels that are freeze-resistant and heat-resistant and have high ultimate tensile strength are desirable in practical applications owing to their potential in designing flexible energy storage devices, actuators, and sensors. Here, a simple method for fabricating ionic liquid (IL)-based click-ionogels using thiol-ene click chemistry under mild condition is reported. These click-ionogels continue to exhibit excellent mechanical properties and resilience after 10,000 fatigue cycles. Moreover, due to several unique properties of ILs, these click-ionogels exhibit high ionic conductivity, transparency, and nonflammability performance over a wide temperature range (-75 degrees to 340 degrees C). Click-ionogel-based triboelectric nanogenerators exhibit excellent mechanical, freeze-thaw, and heat stability. These promising features of click-ionogels will promote innovative applications in flexible and safe device design.
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