Journal
MACROMOLECULES
Volume 52, Issue 20, Pages 7531-7546Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.macromol.9b01127
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Funding
- National Science Foundation [DMR 1407645, DMR 1436201, DMR 1436219, DMR 1535412, DMR 1921835]
- Ministry of Education of the Russian Federation [14.W03.31.0022]
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The current approach to regulating mechanical properties of elastomeric materials is predominately based on the exploratory mixing of different polymers, solvents, and fillers-which is both inflexible in application and imprecise in property control. Here we overview a new materials design approach that harnesses well-defined molecular codes of independently controlled architectural parameters to program grand variation of mechanical phenotypes. This design-by-iarchitecture approach generates a set of universal correlations between the molecular architecture and the physical behavior of elastomers. In turn, this will lead to novel solvent-free materials that closely mimic the mechanical behavior of biological tissues, ranging from soft fat tissue to firm skin, and fundamentally change high-impact technologies such as soft robotics, wearable electronics, and biomedical devices.
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