Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 141, Issue 34, Pages 13346-13351Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.9b07323
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Funding
- MPI fur Kohlenforschung
- SNSF [P2EZP2_175112]
- Spanish Ministerio de Educacion, Cultura y Deporte [FPU15/03940, EST17/00459]
- Swiss National Science Foundation (SNF) [P2EZP2_175112] Funding Source: Swiss National Science Foundation (SNF)
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We report diverse C-N cross-coupling reactions of aryl thianthrenium salts that are formed site-selectively by direct C-H functionalization. The scope of N-nucleophiles ranges from primary and secondary alkyl and aryl amines to various N-containing heterocycles, and the overall transformation is applicable to late-stage functionalization of complex, drug-like small molecules.
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